M. Glässl, A. Barth, K. Gawarecki, P. Machnikowski, M. D. Croitoru, S. Lüker, D. E. Reiter, T. Kuhn, V. M. Axt
We investigate theoretically under which conditions a stable and high-fidelity preparation of the biexciton state in a quantum dot can be realized by means of adiabatic rapid passage in the presence of acoustic phonon coupling. Our analysis is based on a numerically complete real-time path integral approach and comprises different schemes of optical driving using frequency-swept (chirped) pulses. We show that depending on the size of the biexciton binding energy, resonant two-photon excitations or two-color schemes can be favorable. It is demonstrated that the carrier-phonon interaction strongly affects the efficiency of the protocols and that a robust preparation of the biexciton is restricted to positive chirps and low temperatures. A considerable increase of the biexciton yield can be achieved realizing temperatures below 4 K.
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http://arxiv.org/abs/1210.1420
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