Worasom Kundhikanjana, Zhigao Sheng, Yongliang Yang, Keji Lai, Michael A. Kelly, Masao Nakamura, Masashi Kawasaki, Yoshinori Tokura, Qiaochu Tang, Kun Zhang, Xinxin Li, Zhi-Xun Shen
Glassy states are of crucial importance for both fundamental science and applications. Despite being one of the oldest problems, the intriguing dynamics close to the vitrification point are still poorly understood. Part of the difficulty arises from the traditional bulk measurements being hard to interpret. Here, we performed a microscopic study of the strain-induced glassy behavior in epitaxial Pr$_{0.55}$(Ca$_{0.75}$Sr$_{0.25}$)$_{0.45}$MnO$_3$ (PCSMO) thin films using a novel microwave impedance microscopy (MIM). The strong MIM contrast between spatially coexisting ferromagnetic metallic (FM-M) and charge-ordered insulating (CO-I) phases11 reveals the microstructure of the slow relaxation behavior. Randomness of the phase separation from different cooling processes and cross-correlation of time-dependent images provide direct evidence of the non-ergodic and freezing behaviors. Our data also reveal a connection between underlying lattice strains and the glassy kinetics at mesoscopic length and laboratory time scale, demonstrating the strikingly extended hierarchy of scales in glassy physics.
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http://arxiv.org/abs/1306.3065
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